The optimum condition for the removal of MB from aqueous solution under the experimental conditions used in this work was aging time is 30 hours, Thin Film pulling speed is 0.2 mm/s , freeze drying process , pH of 10 and MB concentration of 3 mg/L . It gave maximum adsorption capacity of 20.54 mg/g. The comparative study indicated that powder, fiber and thin film layer could be considered as potential adsorbents, and thin film layer adsorbent as one of the best adsorbents for MB removal from aqueous solutions. This adsorption was single layer adsorption and physic sorption.