Here, we reported the adsorption behavior and mechanism of methyl blue (MB) on the amorphous transitional metal oxide (Fe, Co and Ni oxide) nanoperticles, and we demonstrated that the amorphousization of transitional metal oxide (Fe, Co and Ni oxide) nanoparticles driven by a novel process involving laser irradiation in liquid can create a super adsorption capability for MB, and the maximum adsorption capacity of the fabricated NiO amorphous nanostructure reaches up to 10584.6 mgg-1, the largest value reported to date for all MB adsorbents. The proof-of-principle investigation of NiO amorphous nanophase demonstrated the broad applicability of this methodology for obtaining new super dyes adsorbents.