Titanium-based implants are key weight-bearing materials in biomedical engineering due to their excel-lent bulk mechanical properties and biocompatibility. Designing tissue-material interfaces of titaniumimplants is essential for an increase in osteointegration of engineered implant materials. Surface mor-phology is a crucial determinant in the construction of biocompatible and osteointegrative orthopedic anddental implants. Biomimicry of the structural features of bone, specifically its macro-to-mesoporosity,may enable the bone cells to osteointegrate, attain and maintain a physiological strain level. In this study,the surface chemistry and morphology of commercially pure titanium plates were modified using elec-trochemistry. Titanium oxide substrates were prepared by dual acid polishing and alkaline anodizationusing 0.1 M KOH in an electrochemical cell with a stainless steel cathode and an anodic voltage of 40 V at20◦C for 3 min. FE-SEM characterization revealed macro-mesoporous anodized titania surfaces, whichwere coated by hydroxyapatite using simulated body fluid and pulsed electrochemical deposition at 80◦C,while unprocessed commercially pure titanium surfaces were used as controls. The calcium phosphatedeposit on titania plates was characterized as calcium-deficient carbonated hydroxyapatite using XRD,FTIR and FE-SEM, whereas the deposit on non-porous, non-functionalized titanium surfaces was charac-terized as carbonated apatite. The adhesion strength of the hydroxyapatite coated titania surfaces was38 ± 10 MPa, implying that these surfaces may be suitable for biological and chemical functionalizationof medical implants to tune bioactivity, including delivering drugs.